ENGLISH

Glassy Nuclei in Amorphous Ice: Novel Evidence for the Two-Liquids Nature of Water

By Christina Maria Tonauer

Book information

Publisher
Springer Fachmedien Wiesbaden; Springer Spektrum
Year
2019
ISBN
978-3-658-26323-2;978-3-658-26324-9
Language
english
Format
PDF
Filesize
8 MB (7876852 bytes)
Series
BestMasters
Edition
1st ed.
Pages
XIII, 76\87
Time added
2019-09-18 12:20:48
Chemistry; Physical Chemistry; Inorganic Chemistry

Description

Christina Maria Tonauer finds novel evidence for the first-order nature of the transition between high-density amorphous ice (HDA) and low-density amorphous ice (LDA), supporting water’s liquid-liquid transition scenarios. Pressure-dependent crystallisation experiments of differently prepared expanded high-density amorphous ice samples (eHDA) and subsequent powder x-ray diffraction experiments disclose nucleation of LDA domains in bulk HDA, a typical feature of a first-order transition. The comparison of pressure-dependent crystallisation temperatures of eHDA samples with LDA nuclei and bulk LDA allows the estimation of the Laplace pressure and the size of a LDA nucleus. Front Matter ....Pages I-XIII Introduction (Christina Maria Tonauer)....Pages 1-24 Methods (Christina Maria Tonauer)....Pages 25-28 Experimental section [167] (Christina Maria Tonauer)....Pages 29-56 Discussion [167] (Christina Maria Tonauer)....Pages 57-60 Summary [166] (Christina Maria Tonauer)....Pages 61-62 Back Matter ....Pages 63-76

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